DEVELOPMENT OF LOW TEMPERATURE GLASS CERAMIC FROM LOCAL RAW MATERIALS

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Date
2008-12
Authors
ALI, EDWIN ADOYI
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Abstract
Glass ceramics, a new family of polycrystalline materials produced by the controlled crystallization of glass has many uses cutting across all spheres of life from domestic appliances through medical devices to space exploration. The production process, just like that of other pyrotechnic products, takes a high toll on energy demand as a high temperature process. The best example can be drawn from the US economy where the annual energy bill for the glass industry as a multibillion-dollar industry is put at more than 1.3 billion USD. In the present study, an attempt is made to find alternative route for ceramic glass production in the Nigeria that is cost effective in terms of energy input. In the process, a novel route outside the two usual routes employed in glass ceramic production was adopted in fabricating a product which when subjected to some physical tests showed every attribute of glass ceramics. Although the process, which involved the sintering crystallization of glass and crystalline composites, has no preference to any particular glass composition or crystalline material, a low melting glass composition was used in the experiment to situate the process within the many limitations of the experiment. In this case an ophthalmic glass composition was selected, partially melted at 1200oC, fritted and remixed with a fresh batch and sintered at 1000oC. The percentage water absorption, porosity bulk density and specific gravity were evaluated using by the Archimedes’ Principle (ASTM C373). The evaluation of these properties has a direct bearing to the ultimate characteristics of the glass-ceramic product. The values obtained were 0.176 % for water absorption, 0.268% for porosity, 1.528 for specific gravity and 1.53gcm-3 for density. The density is indicative of a lightweight material relative to the properties of the derivative materials. The XRD analysis shows the main crystalline phase in the material to be cristobalite and nephline. Optical microscopy obtained confirmed the presence of crystalline phases in a glassy matrix, which is conclusive of the fact that the product is indeed glass ceramic. With further improvement the product of the experiment is a candidate for application as an electronic spacer as a lightweight material. However if substitute can be found for the Pb content, which is considered a toxic substance, its future use will extend to utility objects.
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A DISSERTATION SUBMITTED TO THE POSTGRADUATE SCHOOL IN PARTIAL FULFILLMENT OF THE REQUIREMENTS FOR THE AWARD OF THE DEGREE OF DOCTOR OF PHILOSOPHY IN INDUSTRIAL DESIGN (GLASS TECHNOLOGY) DEPARTMENT OF THE INDUSTRIAL DESIGN FACULTY OF SCIENCE AHMADU BELLO UNIVERSITY ZARIA NIGERIA. DECEMBER, 2008
Keywords
DEVELOPMENT,, OF LOW TEMPERATURE,, GLASS,, CERAMIC,, LOCAL RAW MATERIALS
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